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- W1978536441 abstract "A semiempirical formula is derived which governs the electric field dependence of the fluorescence produced upon recombination of geminate ions. The formula is applied to some new data on the fluorescence which follows the ultraviolet irradiation of solutions of N,N,N′,N′-tetramethylparaphenylenediamine (TMPD) in tetramethylsilane and 2,2-dimethylbutane. From the two-parameter-least-squares lines which result from the application of the formula, we determine a number of derived quantities. Among these are Φip the quantum yield for photoionization of TMPD, and P(0,0) the probability of dissociation of the electron–ion pair produced by the photoionization. The values of P(0,0) are found to be nearly equal to the ratio Gfi/(Ggi+Gfi) where Gfi and Ggi are the free ion and geminate ion yields, respectively, obtained in 60Co γ irradiations of the pure solvents. The product of Φip and P(0,0) is Φe0, the free electron quantum yield. The values of Φe0 obtained from the fluorescence measurements are compared with those obtained from separate measurements of the photocurrent. Other quantities derived from the semiempirical formula include the first three moments of a function related to the distribution of electron–ion pair distances in the liquid." @default.
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- W1978536441 date "1981-02-01" @default.
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- W1978536441 title "Semiempirical formula for the electric field dependence of geminate ion recombination fluorescence" @default.
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- W1978536441 doi "https://doi.org/10.1063/1.441311" @default.
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