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- W1978568287 abstract "The vibrationally mediated photodissociation of CS(2)(+) cations via the A(2)Π(u)(ν(1),ν(2),0) state has been studied by means of the velocity map ion imaging technique. The measurements were made with a double resonance strategy. The CS(2)(+) cations were prepared by a (3 + 1) resonance enhanced multiphoton ionization method. The photo-fragment excitation spectrum of S(+) was recorded by scanning the photolysis laser via the A(2)Π(u)(ν(1),ν(2),0) state. By fixing the photolysis laser wavelength at the specific vibrational state, the (1 + 1) photodissociation images of S(+) photofragments from numerous vibrationally mediated states have been accumulated. The translational energy release spectra derived from the resulting images imply that the co-fragments, CS radicals, are both vibrationally and rotationally excited. The one-photon photodissociation without the vibrational state selection has also been performed. Comparing the vibrationally mediated photodissociation with one-photon photodissociation observations, clear evidence of vibrational state control of the photodissociation process is observed." @default.
- W1978568287 created "2016-06-24" @default.
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- W1978568287 date "2012-01-01" @default.
- W1978568287 modified "2023-09-23" @default.
- W1978568287 title "Mode specific photodissociation of CS2+via the A2Πu state: a time-sliced velocity map imaging study" @default.
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- W1978568287 doi "https://doi.org/10.1039/c2cp22385f" @default.
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