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• W1978568638 abstract "Marcus theory has explained how thermal nuclear motions modulate the energy gap between donor and acceptor sites in protein electron transfer reactions. Thermal motions, however, may also modulate electron tunneling between these reactions. Here we identify a new mechanism of nuclear dynamics amplification that plays a central role when interference among the dominant tunneling pathway tubes is destructive. In these cases, tunneling takes place in protein conformations far from equilibrium that minimize destructive interference. As an example, we demonstrate how this dynamical amplification mechanism affects certain reaction rates in the photosynthetic reaction center and therefore may be critical for biological function." @default.
• W1978568638 created "2016-06-24" @default.
• W1978568638 creator A5027249645 @default.
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• W1978568638 date "2000-10-06" @default.
• W1978568638 modified "2023-09-25" @default.
• W1978568638 title "Dynamically Controlled Protein Tunneling Paths in Photosynthetic Reaction Centers" @default.
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• W1978568638 doi "https://doi.org/10.1126/science.290.5489.114" @default.
• W1978568638 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/11021791" @default.
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