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- W1978589905 abstract "Abstract The valence ionization energies and relative intensities of CH 3 N 3 , NCN 3 , cis - and trans -H 2 CCHN 3 , NC-CH 2 -N 3 and CF 3 N 3 are calculated by a many-body Green's function method. Strong correlation effects are observed. As a consequence, it is possible to interpret only the first few lines of the photoelectron spectra in the molecular orbital model. Satellite lines of large relative intensity appear at about 15 eV and are numerous there. The assignment of the spectra at this energy is in general no longer possible in the orbital model, but the many-body calculations permit an analysis. Many-body effects are much stronger for electron ejection from orbitals localized on the N 3 (and the CN) group than from orbitals localized on the CH 3 or CF 3 group. The lowest ionization energies of cis - and trans -vinylazide are very close to each other and from a calculation of the lower ionization energies it is not possible to distinguish between the two isomers." @default.
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- W1978589905 date "1989-01-01" @default.
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- W1978589905 title "Many-body effects in the ionization spectra of azides" @default.
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- W1978589905 doi "https://doi.org/10.1016/0368-2048(89)80015-5" @default.
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