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- W1978726114 abstract "We produce a cool pulsed supersonic molecular beam of CaF radicals essentially without recourse to pumping. The radicals are generated by laser ablating a solid precursor target in a small ablation cell of volume of about 0.01 cm3. The target is ablated through a 750 μm orifice by a pulsed Nd:YAG laser. The ablation plume supersonically expands into a vacuum chamber and cools the initially hot CaF molecules seeded in it. We enhance the supersonic character of the expansion by feeding into the ablation cell about 10 Torr of He, Ar, or Xe carrier gas. The CaF molecules are probed by time-dependent laser absorption spectroscopy. With a Xe carrier, about 1012 CaF molecules are found to be seeded in a single pulse and cooled down to a terminal translational temperature of about 140 K. We expect that a wide variety of species, including highly unstable ones, will be amenable to forming such a cool intense molecular microbeam, to the benefit of spectroscopy, reaction dynamics, and microfabrication." @default.
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- W1978726114 date "2003-12-22" @default.
- W1978726114 modified "2023-10-17" @default.
- W1978726114 title "Cool pulsed molecular microbeam" @default.
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- W1978726114 doi "https://doi.org/10.1063/1.1630836" @default.
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