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• W1978826551 endingPage "9267" @default.
• W1978826551 startingPage "9254" @default.
• W1978826551 abstract "There are three alternative perturbation procedures which are equivalent when considering the contribution of the spin-orbit (SO) mechanism to the spin-Hamiltonian parameters of $^{6}mathrm{state}$ ions. We show that the study of the uniaxial stress on the zero-field splitting is an effective way of identifying the most important contributor among the various mechanisms leading to the $^{6}mathrm{state}$ splitting. Calculations are carried out for ${mathrm{Mn}}^{2+}$ and ${mathrm{Fe}}^{3+}$-doped MgO and CaO crystals, indicating the SO mechanism to be predominant in the systems. The importance of utilizing the appropriate crystal-field model is stressed, and the observed axial term D of ${mathrm{Fe}}^{3+}$ and ${mathrm{Mn}}^{2+}$ ions at the tetrahedral and octahedral sites in several garnets are well explained by the SO mechanism, with the aid of the superposition model of the crystal field. The superposition model of the spin Hamiltonian proposed by Newman and Urban is shown to be capable of reaching results identical with those of the SO and other microscopic mechanisms. Illustrations are given indicating that the investigation of the intrinsic parameter and the power-law exponent of the superposition model is helpful in the identification of the dominant one among the mechanisms." @default.
• W1978826551 created "2016-06-24" @default.
• W1978826551 creator A5020494190 @default.
• W1978826551 creator A5027134071 @default.
• W1978826551 date "1988-06-01" @default.
• W1978826551 modified "2023-09-26" @default.
• W1978826551 title "Spin-Hamiltonian parameters of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi mathvariant=normal>state</mml:mi></mml:mrow><mml:mprescripts /><mml:mrow /><mml:mrow><mml:mn>6</mml:mn></mml:mrow><mml:mrow /><mml:mrow /></mml:mmultiscripts></mml:mrow></mml:math>ions" @default.
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• W1978826551 doi "https://doi.org/10.1103/physrevb.37.9254" @default.
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