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- W1979017665 abstract "Abstract The standard analysis of light-scattering experiments, which presumes single scattering, cannot be applied in highly turbid systems because of the presence of multiply scattered light. Cross-correlation techniques, however, enable to determine the intensity and the correlation function of singly scattered light even in the presence of multiple scattering. We present here a novel theoretical assessment of the influence of experimental conditions (intensity distribution of the laser beam, aperture of the fiber optics, scattering geometry) on the scattering intensity, and on the amplitude of the cross-correlation function for the three-dimensional (3D) coding cross-correlation experiment. The theory makes use of the rotation operator when transforming vectors and the coefficient matrices of the Gauss functions which represent the intensity distribution of the laser and the aperture function of the fiber optics. Rather simple analytical results are obtained for the scattering volume, the polarization of the scattered light, the overlap volume and the amplitude of the correlation function in the cross-correlation experiment. The effects of misalignment are assessed in a general way. The optimal setup is characterized by a small incidence angle of the laser beams (≈ 1°), equality of the intensities of the incident beams, and by equality of the widths of the laser beams of the apertures of the detection systems. Under those conditions the amplitude of the intensity cross-correlation function can approach the optimum of 1 4 for 90° scattering and shows a plateau in a wide region of the goniometer angles." @default.
- W1979017665 created "2016-06-24" @default.
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- W1979017665 date "2002-05-01" @default.
- W1979017665 modified "2023-09-27" @default.
- W1979017665 title "Application of the rotation operator in the design of light-scattering experiments" @default.
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- W1979017665 doi "https://doi.org/10.1016/s0167-7322(01)00322-1" @default.
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