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- W1979092279 abstract "Dynamic properties of a binary Lennard-Jones mixture at various temperatures and two densities are studied using a molecular dynamics computer simulation starting from mixed and separated initial configurations. After deriving an analytical correction term for finite size effects, the rate of separation is determined as a function of temperature, which is influenced by two counteracting trends: at higher particle velocities demixing becomes faster, but with increasing temperature the separated state becomes less stable. At both densities studied, we observe an increase in the rate of separation with increasing temperature. In a second step, a small number of a third type of particle representing a crude model of an amphiphilic molecule is added and the results are compared with those of the binary mixture case. Owing to a dip in the density at the binary fluid interface, the amphiphilic molecules collect in a slit and as a result, no effect on the separation behaviour of the system is observed. At those temperatures for which the separated configuration is stable, the typical behaviour of the individual particle is analysed." @default.
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- W1979092279 date "1994-08-10" @default.
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- W1979092279 title "Molecular dynamics study of the mixing and demixing of a binary Lennard-Jones fluid" @default.
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- W1979092279 doi "https://doi.org/10.1080/00268979400100744" @default.
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