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- W1979112041 abstract "We report a procedure that for the first time allows the quantitative determination of the lengthening δr of the HF bond on formation of an isolated hydrogen-bonded dimer B···HF. We show how δr can be obtained from the ground-state hyperfine coupling constants X (D nuclear quadrupole) and D HF (H, F nuclear spin to nuclear spin), which are available from the rotational spectra of the molecules B···H(D)F. We establish the values of δr for the series of heterodimers B···HF where B = Ar, Kr, Xe, N 2 , CO, H 2 S, HCN, CH 3 CN and H 2 O. The values of δr are zero for the first three members of this series and then 0.001, 0.007, 0.010, 0.014, 0.016 and 0.015 Å, respectively (1 Å = 10 -1 nm = 10 -10 m). It is found that δr is a monotonically increasing function of the hydrogen-bond stretching force constant k σ , which is taken as a convenient measure of the hydrogen bond strength." @default.
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- W1979112041 date "1986-03-08" @default.
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- W1979112041 title "The lengthening of the HF bond on formation of heterodimers B • • • HF: determination and dependence on the strength of the hydrogen bond" @default.
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- W1979112041 doi "https://doi.org/10.1098/rspa.1986.0020" @default.
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