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• W1979191736 abstract "The reactive scattering of formic acid from Ni(110) was studied over the temperature range of 175–920 K with MBRS in the millisecond time region by employing a modulation frequency of 36.8 Hz. The steady-state carbon and oxygen composition of the surface varied over the range of temperatures studied. For beam fluxes of 1013 molecules/cm2 sec the onset of decomposition on the steady-state surface occurred at 300 K. By 400 K decomposition was essentially complete, and the products CO2, CO, H2 and H2O were detected. All reaction events were prceded by a common step, and the products were then produced by a series/parallel mechanism. The rate constants measured for H2 and H2O formation indicated stringent limitations on the efficiency of second-order collisions on the surface for producing gaseous products. This study illustrates the use of MBRS for surface reaction mechanistic studies in the millisecond time scale." @default.
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• W1979191736 date "1977-06-01" @default.
• W1979191736 modified "2023-09-23" @default.
• W1979191736 title "The kinetics and mechanism of catalytic reactions by molecular beam relaxation spectroscopy: HCOOH decomposition" @default.
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• W1979191736 doi "https://doi.org/10.1016/0039-6028(77)90308-9" @default.
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