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• W1979331603 abstract "Applying a recently developed micellar technique, ordered arrays of gold nanoparticles with narrow size distributions were deposited onto thin Nb(110) films covered by an ultrathin ${mathrm{Al}}_{2}{mathrm{O}}_{3}$ layer of thickness $ensuremath{sim}1phantom{rule{0.3em}{0ex}}mathrm{nm}$ serving as tunneling barrier. Analyzing these particles by scanning tunneling microscopy and spectroscopy at room temperature revealed Coulomb blockade (CB) effects with charging energies in the range $0.2--1.5phantom{rule{0.3em}{0ex}}mathrm{eV}$. Relevant CB parameters of individual nanoparticles, which are clearly separated from their neighbors, could be determined quantitatively by fitting experimentally obtained current-voltage curves to orthodox theory. In this way, an almost linear relation between the total capacitance of the CB system and the particle size is found as expected for a simple free sphere model with an effective dielectric constant. Though the agreement between orthodox theory and experiment in general is satisfying, there are also some significant deviations such as non-Ohmic behavior of the tunneling barriers, a strong dependence of the charging on the lateral position of the tunneling tip with respect to a single particle, and an unexpected heating effect possibly due to the long dwell time of the charge carriers on the islands." @default.
• W1979331603 created "2016-06-24" @default.
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• W1979331603 date "2007-02-07" @default.
• W1979331603 modified "2023-09-23" @default.
• W1979331603 title "Dynamic charging at room temperature of Au nanoparticles prepared by a micellar technique" @default.
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• W1979331603 doi "https://doi.org/10.1103/physrevb.75.085407" @default.
• W1979331603 hasPublicationYear "2007" @default.
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