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- W1979381519 abstract "We investigate the resonance Raman scattering of finite and infinite polyenes. The connection between the vibronic picture of Raman scattering and the third order perturbation approach normally used in solid state physics for infinite systems is clarified. Starting from the Kramers–Heisenberg–Dirac formula for the Raman scattering, we derive expressions for the Condon and Herzberg–Teller terms for chains from N=2 (a simple two-level system) to N=∞ (a two-band system) by using the standard vibronic picture. Close to resonance the Condon term dominates and converges to the usual solid state result. In the off-resonance region, the Herzberg–Teller term is comparable to the Condon term for both the small molecule and the solid state system." @default.
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- W1979381519 date "1995-03-08" @default.
- W1979381519 modified "2023-09-26" @default.
- W1979381519 title "Theory of resonance Raman scattering for finite and infinite polyenes" @default.
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- W1979381519 doi "https://doi.org/10.1063/1.469472" @default.
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