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- W1979415833 abstract "A tandem cross metathesis (CM)--ring-closing metathesis (RCM) sequence to form cyclic siloxanes is reported. This new enyne metathesis platform expands the scope and utility of the regio- and stereoselective cross metathesis reaction between silylated alkynes and terminal alkenes. The initial cross metathesis was directed to occur on the alkyne by employing sterically hindered mono-, di-, and trisubstituted alkenes tethered to the alkyne via silyl ether. The regio- and stereoselectivity feature of the initial CM step in this tandem CM-RCM process is identical to that of the CM reactions of silylated alkynes and alkenes. This tandem sequence provides both synthetically useful silylated 1,3-diene building blocks and insights into the reaction mechanism of the enyne metathesis reaction." @default.
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- W1979415833 date "2005-06-14" @default.
- W1979415833 modified "2023-09-23" @default.
- W1979415833 title "Tandem Sequence of Cross Metathesis−Ring-Closing Metathesis Reaction of Alkynyl Silyloxy-Tethered Enynes" @default.
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- W1979415833 doi "https://doi.org/10.1021/ja0520159" @default.
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