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- W1979451505 abstract "In a study of non-equilibrum ionization in shock layers, the chemical system (1) O2 + X ⇌ O + O + X (2) O + N2 ⇌ N + NO (3) O + NO ⇌ N + O2 (4) N + O ⇌ NO+ + e was adopted as the simplest system which could reasonably be used in calculation of ionization rates and times. Use of the rates of the individual reactions permitted the calculations of the electron density and other concentrations in the plasma sheath as functions of time. Important quantities in such calculations are the reaction rate constants which, together with the concentrations, determine the actual rates. Values of these constants are greatly in doubt. A programme was set up to determine the effect of inaccuracies in these values. Each pair of rate constants was changed individually and the effect on each concentration-time curve was noted. Large effects were found. In one typical case, a change of one order of magnitude in the rate constant of the O2 dissociation changed the electron density after about two msec by a factor of about 200. Changes of other rate constants by an order of magnitude changed the overall rate of ionization by lesser, but still serious, factors. It is therefore concluded that non-equilibrium electron density calculations are extremely dependent on the values of the rate constants and precise values are needed." @default.
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- W1979451505 date "1961-06-01" @default.
- W1979451505 modified "2023-09-26" @default.
- W1979451505 title "The effect of errors in rate constants on non-equilibrium shock layer electron density calculations" @default.
- W1979451505 doi "https://doi.org/10.1016/0032-0633(61)90006-x" @default.
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