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• W1979486514 endingPage "20703" @default.
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• W1979486514 abstract "A detailed mechanism for isoprene photooxidation is developed that includes the recent developments on each of isoprene's atmospherically important reactions: O[sub 3], OH, O([sup 3]P), and NO[sub 3] as well as the OH reactions of methacrolein and methyl vinyl ketone. The mechanism also attempts to account for the gaps in the product distributions for a few reactions. The CO yield from isoprene oxidation in the presence of NO[sub x], more than about 50 ppt, is calculated as about 3.4. The mechanism is tested against chamber data that include a range of mixtures of the primary oxidants, isoprene concentrations, and hydrocarbon/NO[sub x] ratios. It performs well under conditions where the OH and O([sup 3]P) reactions dominate the predicts peak O[sub 3] concentrations within about 25% under all conditions. The mechanism underpredicts methyl vinyl ketone yields as well as O[sub 3] levels under conditions of low available NO[sub x]. Sensitivity of the mechanism to assumptions about the NO[sub 3] and O[sub 3] reactions are examined, and possible sources of the discrepancies are discussed. A condensed mechanism is developed and compared to the explicit mechanism. 48 refs., 6 figs., 3 tabs." @default.
• W1979486514 created "2016-06-24" @default.
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• W1979486514 date "1992-01-01" @default.
• W1979486514 modified "2023-10-14" @default.
• W1979486514 title "Development and evaluation of a photooxidation mechanism for isoprene" @default.
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• W1979486514 doi "https://doi.org/10.1029/92jd01914" @default.
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