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- W1979489969 abstract "Abstract Potentiostatic anodic polarization studies have been conducted in a J-13 simulated nuclear waste repository environment, where the environment was allowed to evaporate to dryness followed by rehydration prior to polarization. The behavior noted for Type 316L stainless steel, AISI 1020 carbon steel, Hastelloy C22 and platinum was compared with that noted previously for a non-baked simulate. The anodic dissolution characteristics of Type 316L stainless steel in environments containing 1000X Cl − J-13 depend markedly on whether the solution is merely a mixture of virgin chemicals or a mixture that has been evaporated to dryness, baked and rehydrated to the same volume. In the non-evaporated environment Type 316L stainless steel pitted severely, and in the evaporated/rehydrated environment a non-corroding type of behavior was observed along with the precipitation of a dense scale. The same differing behavior was observed for Hastelloy C22 along with scale formation in the evaporated solution. The polarization curves for carbon steel and platinum were the same as those noted for 316L and Hastelloy C22 (including the deposition of scale), when conducted in the evaporated/rehydrated environment. X-Ray diffraction studies indicated that the scale produced in all tests conducted on evaporated/rehydrated solutions was calcium carbonate. Based on the qualitatively similar polarization characteristics of materials having such widely differing corrosion properties, it is concluded that the major factor controlling the anodic charge transfer reaction under these conditions is the formation of a calcium carbonate scale. These observations make it clear that future studies in Tuff type environments should, at least in part, be focussed on material performance in solutions produced by an evaporation/rehydration cycle similar to that anticipated in practice on the walls of buried canisters." @default.
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- W1979489969 date "1993-03-01" @default.
- W1979489969 modified "2023-09-27" @default.
- W1979489969 title "Some observations on the mechanism of corrosion to be encountered in nuclear waste repositories located in tuffaceous rock" @default.
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- W1979489969 doi "https://doi.org/10.1016/0010-938x(93)90115-w" @default.
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