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• W1979541462 abstract "Abstract A new oxide of stoichiometry HoFeMnO 5 has been obtained by replacing Mn 3+ cations by Fe 3+ in the parent oxide HoMn 2 O 5 . The crystallographic and magnetic structures have been analyzed by neutron powder diffraction (NPD), which complements susceptibility and magnetization measurements. HoFeMnO 5 is orthorhombic, belonging to the Pbam space group like the parent compound. The crystal structure contains infinite chains of edge‐sharing Mn 4+ O 6 octahedra, interconnected by dimer units of Fe 3+ O 5 square pyramids. In comparison with HoMn 2 O 5 , containing elongated Mn 3+ O 6 pyramids, the Fe 3+ O 5 units are flattened. The magnetization measurements show that HoFeMnO 5 presents a long‐range magnetic order below T C ≈ 153 K. An NPD study shows that HoFeMnO 5 adopts a collinear ferrimagnetic structure: each of the Mn 4+ and Fe 3+ sublattices are ferromagnetically coupled, and the coupling between the two sublattices is antiferromagnetic; the magnetic moments are oriented along the c direction. The Ho 3+ cations also order below T C , but with a very small magnetic moment; the Ho 3+ moments are parallel to the Fe 3+ magnetic sublattice. At T = 2.7 K, the ordered magnetic moments for the Mn 4+ , Fe 3+ and Ho 3+ ions are 1.31(6), 3.20(10) and 0.36(7) μ B , respectively. In comparison with ErFeMnO 5 , where Er 3+ cations are fully ordered at low temperatures, in HoFeMnO 5 there is a frustration concerning the long‐range order of the Ho 3+ cations, which remain virtually paramagnetic over the whole temperature range.(© Wiley‐VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2007)" @default.
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• W1979541462 date "2007-04-20" @default.
• W1979541462 modified "2023-10-18" @default.
• W1979541462 title "Synthesis and Study of the Crystallographic and Magnetic Structure of HoFeMnO ₅" @default.
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• W1979541462 doi "https://doi.org/10.1002/ejic.200601144" @default.
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