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- W1979625452 abstract "Benzyl and benzyl-α-d2 radicals are produced by the ArF laser (193 nm) photolysis of benzylchloride and benzylchloride-α-d2, respectively, in a supersonic free jet. The spectroscopy of the D1 1 2A2–D0 1 2B1 transition of these radicals is studied by means of the laser induced fluorescence (LIF) method. LIF excitation spectra show well resolved but unusual vibrational structure. The assignments of vibronic bands have been carried out on the basis of dispersed spectra from the single vibronic level (SVL) and transition band types derived from rotational analysis of high resolution LIF excitation spectra. The intensity anomaly of the vibronic bands in the excitation spectra is interpreted as the breakdown of the accidental forbidden character of the D1–D0 and D2–D0 electronic transitions, whose mechanism will be discussed in terms of vibronic coupling." @default.
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- W1979625452 date "1992-03-15" @default.
- W1979625452 modified "2023-09-27" @default.
- W1979625452 title "Jet spectroscopy of benzyl and benzyl-α-<i>d</i>2" @default.
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- W1979625452 doi "https://doi.org/10.1063/1.462815" @default.
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