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• W1979700970 abstract "We have measured the high-resolution infrared spectrum of the radical NO in the $^{2}ensuremath{Pi}_{1/2}$ state in superfluid helium nanodroplets. The features are attributed to the $ensuremath{Lambda}$-doubling splitting and the hyperfine structure. The hyperfine interaction is found to be unaffected by the He solvation. For the $ensuremath{Lambda}$-doubling splitting, we find a considerable increase by 55% compared to the gas phase. This is explained by a confinement of the electronically excited NO states by the surrounding He. The rotational level spacing is decreased to 76% of the gas phase value. The IR transition to the $J=1.5$ state is found to be homogeneously broadened. We attribute both observations to the coupling between the molecular rotation and phonon/roton excitations in superfluid $^{4}mathrm{He}$ droplets." @default.
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• W1979700970 date "2005-11-14" @default.
• W1979700970 modified "2023-10-03" @default.
• W1979700970 title "High-Resolution Spectroscopy of NO in Helium Droplets: A Prototype for Open Shell Molecular Interactions in a Quantum Solvent" @default.
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• W1979700970 doi "https://doi.org/10.1103/physrevlett.95.215301" @default.
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