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• W1979968163 abstract "Cyanide-bridged trinuclear complexes containing square-planar platinum at the center were synthesized and identified by structure determinations. Their chemical building blocks were cis- and trans-PtL2X2, Cp(dppe)FeX, Cp(PPh3)2RuX (with X = Hal or CN), Pt(CN)42-, and Fe(CN)63-. Several of the intermediate dinuclear complexes were isolated and used for reference purposes. The molecular structures, the ν(CN) IR data, the cyclic voltammograms, and the UV−vis−near-IR spectra were used to probe the effects of the geometry at platinum (cis vs trans), of cyanide−isocyanide isomerism (Pt(CN)2 vs Pt(NC)2), of the nature and ligation of the terminal metals (Fe vs Ru), and of one- or two-electron oxidation. The redox properties and the observed intervalence transfers indicate that there is electronic communication between the outer metal atoms along the linear M−CN chains containing trans-configured platinum, but not along the bent chains containing cis-configured platinum." @default.
• W1979968163 created "2016-06-24" @default.
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• W1979968163 date "1999-06-01" @default.
• W1979968163 modified "2023-10-17" @default.
• W1979968163 title "Linear and Bent M(μ-CN)Pt(μ-CN)M Chains: Probes for Remote Metal−Metal Interactions" @default.
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• W1979968163 doi "https://doi.org/10.1021/ic981384l" @default.
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