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• W1980660215 abstract "Abstract A sequential stimulated Raman adiabatic passage (STIRAP) approach is applied to the laser control of internal double proton transfer of a porphyrin derivative. The potential energy surfaces describing the motion of the two protons are evaluated from the density functional theory (DFT) calculation; the minimum‐energy conformers obtained are classified as the trans ‐ and cis ‐forms. It is shown that the STIRAP pulse sequence induces the transition from the most stable trans ‐form to the other trans ‐form via the cis ‐intermediate state on the picosecond time scale. The influence of laser intensity on the STIRAP process of the double proton transfer is discussed. © 2005 Wiley Periodicals, Inc. Int J Quantum Chem, 2005" @default.
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• W1980660215 date "2005-01-01" @default.
• W1980660215 modified "2023-10-16" @default.
• W1980660215 title "Laser control of proton motion in porphyrin derivative" @default.
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• W1980660215 doi "https://doi.org/10.1002/qua.20443" @default.
• W1980660215 hasPublicationYear "2005" @default.
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