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- W1980741566 abstract "In a dilute solution of large polymers, each polymer shrinks when shorter polymers of different species are added, provided that the molecular interaction between the polymers of the two kinds is repulsive. The existence of a sharp transition of the large polymer from an extended random coil to a compact globule is examined in a statistical mechanical way. We show that a first-order-like sharp transition induced by the existence of the smaller polymers takes place under the conditions such that (i) the intermolecular interaction is sufficiently strong compared with the intramolecular interaction between the segments in a large polymer, (ii) the degree of polymerization (DP) of the large polymer is much larger than that of the smaller polymers. The critical concentration of the smaller polymers, above which the large polymer collapses to a closely packed globule, is shown to be inversely proportional to their DP. Detailed numerical analyses on a model system are presented." @default.
- W1980741566 created "2016-06-24" @default.
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- W1980741566 date "1985-03-01" @default.
- W1980741566 modified "2023-09-26" @default.
- W1980741566 title "The polymer‐induced coil–globule transition" @default.
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- W1980741566 doi "https://doi.org/10.1063/1.448291" @default.
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