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• W1980999615 abstract "Six internal rotation/vibration bands of ArH2O are observed in a slit supersonic expansion via direct absorption of a tunable diode laser in the v2 bend region of H2O. The spectra obtained for the ortho H2O manifold are well represented by a pseudodiatomic model with nearly free internal rotation of the H2O subunit. By way of contrast, the para bands show significant mixing between the internal rotor and stretch states, indicative of strong angular-radial coupling in the intermolecular potential. The spectra for the para Ar–H2O species can be deperturbed based on a three state Coriolis plus angular-radial coupling model which includes microwave, far-ir and near-ir data. The results indicate a redshift of ≈0.58 cm−1 upon bend excitation of the H2O subunit, and in general rather modest changes in the excited state intermolecular potential from the ground state potential. No indication of predissociation broadening is found, and the instrument-limited linewidths place a lower limit on the vibrational lifetime in the excited state of τ⩾7.2(6) ns." @default.
• W1980999615 created "2016-06-24" @default.
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• W1980999615 date "1997-02-22" @default.
• W1980999615 modified "2023-10-07" @default.
• W1980999615 title "High resolution mid-infrared spectroscopy of ArH2O: The <i>v</i>2 bend region of H2O" @default.
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• W1980999615 doi "https://doi.org/10.1063/1.473051" @default.
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