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- W1981044933 abstract "Abstract A novel approach to the growth of defect-free epitaxial films of group-III nitrides is being developed with the help of ab initio molecular orbital (MO) methods. Usage of a molecular beam of dialkyl group-III nitrene (characterized from the theoretical point of view not only by two unpaired electrons almost localized at the nitrogen atom but also by the covalently bound pair of one group-III and one nitrogen atom) is advantageous to the low-temperature growth of stoichiometric group-III nitride. Dialkyl group-III nitrene beam can be obtained by photo-dissociation of energetic compound beams (PDECB) using dialkyl group-III azide as source material. Post-SCF ab initio MO methods were applied in this study to screening tests of the organometallic azides suitable as PDECB source compound. Also attempted was clarification of the key points to optimize the growth conditions in terms of the surface chemical reactions involved in homoepitaxial growth of cubic group-III nitride under supply of dimethylaluminumnitrene ((CH3)2AlN) or dimethylgalliumnitrene ((CH3)2GaN)." @default.
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- W1981044933 date "2003-02-01" @default.
- W1981044933 modified "2023-09-26" @default.
- W1981044933 title "Predictive use of ab initio MO methods in PDECB-based approach to low-temperature epitaxy of stoichiometric group-III nitrides" @default.
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- W1981044933 doi "https://doi.org/10.1016/s1369-8001(03)00084-2" @default.
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