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- W1981124443 endingPage "284101" @default.
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- W1981124443 abstract "Atomistic molecular dynamics simulations have been carried out to understand the effect of the symmetry of cations on the microscopic organization of ionic liquids near a charged mica surface. Ionic liquids with a 1,3-alkylimidazolium ([CnCmim]+) cation and a bis(trifluoromethylsulfonyl)imide ([NTf2]−) anion were investigated. Apart from symmetry, the length of the alkyl group attached to the cation is found to crucially determine the ion structure near the solid surface. In the first adsorbed layer, the ring planes of cations with shorter alkyl groups (less than four carbon atoms) are oriented either parallel or perpendicular to the surface. However, cations with longer alkyl tails are exclusively observed to have their ring planes parallel to the mica surface. The alkyl groups too show a similar dependence of their orientation on the tail length. Further, symmetric cations with alkyl groups of intermediate length are more highly structured at the interface than their asymmetric counterparts." @default.
- W1981124443 created "2016-06-24" @default.
- W1981124443 creator A5013255727 @default.
- W1981124443 creator A5028361145 @default.
- W1981124443 date "2014-06-12" @default.
- W1981124443 modified "2023-09-24" @default.
- W1981124443 title "Effect of cation symmetry on the organization of ionic liquids near a charged mica surface" @default.
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- W1981124443 doi "https://doi.org/10.1088/0953-8984/26/28/284101" @default.
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