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• W1981166501 abstract "Peroxycarboxylic nitric anhydrides (PANs) have long been recognized as important trace gas constituents of the troposphere. Here, we describe a blue diode laser thermal dissociation cavity ring-down spectrometer for rapid and absolute measurements of total peroxyacyl nitrate (∑PAN) abundances at ambient concentration levels. The PANs are thermally dissociated and detected as NO2, whose mixing ratios are quantified by optical absorption at 405 nm relative to a reference channel kept at ambient temperature. The effective NO2 absorption cross-section at the diode laser emission wavelength was measured to be 6.1 × 10−19 cm2 molecule−1, in excellent agreement with a prediction based on a projection of a high-resolution literature absorption spectrum onto the laser line width. The performance, i.e., accuracy and precision of measurement and matrix effects, of the new 405 nm thermal dissociation cavity ring-down spectrometer was evaluated and compared to that of a 532 nm thermal dissociation cavity ring-down spectrometer using laboratory-generated air samples. The new 405 nm spectrometer was considerably more sensitive and compact than the previously constructed version. The key advantage of laser thermal dissociation cavity ring-down spectroscopy is that the measurement can be considered absolute and does not need to rely on external calibration." @default.
• W1981166501 created "2016-06-24" @default.
• W1981166501 creator A5038087514 @default.
• W1981166501 creator A5087098755 @default.
• W1981166501 date "2010-07-15" @default.
• W1981166501 modified "2023-09-27" @default.
• W1981166501 title "Absolute Measurements of Total Peroxy Nitrate Mixing Ratios by Thermal Dissociation Blue Diode Laser Cavity Ring-Down Spectroscopy" @default.
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• W1981166501 doi "https://doi.org/10.1021/ac101441z" @default.
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