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• W1981176260 endingPage "104303" @default.
• W1981176260 startingPage "104303" @default.
• W1981176260 abstract "Multichannel quantum-defect theory (MQDT) is used to calculate the electron binding energies of np Rydberg states of H2, HD, and D2 around n = 60 at an accuracy of better than 0.5 MHz. The theory includes the effects of rovibronic channel interactions and the hyperfine structure, and has been extended to the calculation of the asymmetric hyperfine structure of Rydberg states of a heteronuclear diatomic molecule (HD). Starting values for the eigenquantum-defect parameters of MQDT were extracted from ab initio potential-energy functions for the low-lying p Rydberg states of molecular hydrogen and subsequently refined in a global weighted fit to available experimental data on the singlet and triplet Rydberg states of H2 and D2. The electron binding energies of high-np Rydberg states derived in this work represent important quantities for future determinations of the adiabatic ionization energies of H2, HD, and D2 at sub-MHz accuracy." @default.
• W1981176260 created "2016-06-24" @default.
• W1981176260 creator A5012920311 @default.
• W1981176260 creator A5020330910 @default.
• W1981176260 creator A5059729730 @default.
• W1981176260 date "2014-03-14" @default.
• W1981176260 modified "2023-09-30" @default.
• W1981176260 title "Determination of the binding energies of the <i>np</i> Rydberg states of H₂, HD, and D₂ from high-resolution spectroscopic data by multichannel quantum-defect theory" @default.
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• W1981176260 doi "https://doi.org/10.1063/1.4866809" @default.
• W1981176260 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24628165" @default.
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