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• W1981366057 abstract "Surface-enhanced Raman spectroscopy (SERS) is a known approach for detecting trace amounts of molecular species. Whereas SERS measurements have focused on enhancing the signal for sensing trace amounts of a chemical moiety, understanding how the substrate alters molecular Raman spectra can enable optical probing of analyte binding chemistry. Here we examine binding of trans-1,2-two(4-pyridyl) ethylene (BPE) to Au surfaces and understand variations in experimental data that arise from differences in how the molecule binds to the substrate. Monitoring differences in the SERS as a function of incubation time, a period of several hours in our case, reveals that the number of BPE molecules that chemically binds with the Au substrate increases with time. In addition, we introduce a direct method of accessing relative chemical enhancement from experiments that is in quantitative agreement with theory. The ability to probe optically specific details of metal/molecule interfaces opens up possibilities for using SERS in chemical analysis." @default.
• W1981366057 created "2016-06-24" @default.
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• W1981366057 date "2012-05-07" @default.
• W1981366057 modified "2023-09-25" @default.
• W1981366057 title "Harnessing Chemical Raman Enhancement for Understanding Organic Adsorbate Binding on Metal Surfaces" @default.
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• W1981366057 doi "https://doi.org/10.1021/jz300374d" @default.
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