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- W1981511373 abstract "We report the first observation of homogeneous organometallic photocatalysis in the gas phase. Gaseous mixtures of iron pentacarbonly with 1-pentene and hydrogen for hydrogenation (with accompanying isomerization) are irradiated with the pulsed output of a N2 (337 nm) or XeF (351 nm) excimer laser. We observe quantum yields, calculated as number of conversions per photon absorbed, as high as 400 for isomerization and 18 for hydrogenation. Kinetic and spectroscopic evidence suggest that the photocatalytic mechanisms operating in the gas phase closely parallel those of the corresponding, better characterized liquid phase systems. (AIP)" @default.
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- W1981511373 date "1982-10-01" @default.
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- W1981511373 title "Laser photocatalytic isomerization and hydrogenation of olefins in the gas phase" @default.
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- W1981511373 doi "https://doi.org/10.1063/1.444244" @default.
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