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- W1981523055 abstract "The disordering mechanisms which characterize the pretransitional states of a polymethylene chain inserted in a host material are studied with statistical mechanics. While the intramolecular conformational energy of the chain is chosen according to Flory’s theory, the interaction with the host material is modeled in terms of a given external potential. The competition between end-gauche and kink formation is in particular examined: it is shown that chain-end distorsions are initially favored and, with increasing temperature, kink formation and longitudinal translation of the molecular chain sustain the disordering process. The results are compared with the experimental data from vibrational spectroscopy." @default.
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- W1981523055 date "1987-02-01" @default.
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- W1981523055 title "Disordering mechanisms in polymethylene molecules: A chain in a channel" @default.
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- W1981523055 doi "https://doi.org/10.1063/1.452195" @default.
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