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- W1981544649 abstract "A treatment of molecular collision broadening employing the distorted-wave (DW) approximation for the disentanglement of the coupled scattering equations for anisotropic potentials is developed. Calculations of the rotational and vibration–rotation line-shape parameters, for HCl perturbed by Ar, have been performed within the framework of a model potential. The extension to realistic potentials of the DW method, in a DW–WKB version and in the classical-path limit of the DW–WKB approximation, is discussed. For all but the lightest collision couples, the DW–WKB approximation emerges as a method which combines accuracy in the discription of the molecular interaction with relative computational ease; for massive systems, the DW–WKB method can be taken to the classical-path limit with no loss in accuracy. In either of these versions, the DW–WKB approach constitutes a practicable avenue which promises accurate predictions of molecular line shifts and widths." @default.
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- W1981544649 date "1968-05-15" @default.
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- W1981544649 title "Rotational and Vibration–Rotation Line Shifts and Widths. Distorted-Wave Approximation" @default.
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- W1981544649 doi "https://doi.org/10.1063/1.1668010" @default.
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