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- W1981782944 abstract "The oxidation of ethylene oxide on polycrystalline Ag films supported on stabilized zirconia was studied in a CSTR at atmospheric pressure and temperatures between 250 and 400 °C. The new technique of solid electrolyte potentiometry (SEP) was used to monitor the chemical potential of oxygen adsorbed on the metal catalyst. To this end the silver film catalyst also served as one of the electrodes of a solid electrolyte oxygen concentration cell and the open-circuit emf of the cell was monitored during reaction. It was found that the steady-state surface oxygen activity αo is given by a0 = PO212/(1 + KETOXPETOX2), with KETOX = 3.3 · 10−5 exp (10,600T). This equation as well as the kinetics can be explained in terms of a simple reaction mechanism." @default.
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- W1981782944 date "1980-07-01" @default.
- W1981782944 modified "2023-10-16" @default.
- W1981782944 title "Solid electrolyte aided study of the ethylene oxide oxidation on silver" @default.
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- W1981782944 doi "https://doi.org/10.1016/0021-9517(80)90475-3" @default.
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