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• W1981845529 abstract "Sodium formate neutral aqueous solutions saturated with N2O were studied by pulse radiolysis techniques from room temperature to 400 °C. The absorption spectra of CO2− show a red shift from λmax=235 nm at 25 °C to 280 nm at 400 °C. The second-order decay of CO2− is not monotonically temperature-dependent: the rate constant (2k/ε) slightly increases with temperature up to 200 °C, then decreases to a valley at 300 °C, and it sharply increases again for temperature >350 °C. Gε(CO2−) increases with temperature from room temperature to 400 °C. Significant density effect on Gε(CO2−) is found at 400 °C. Assumed ε(CO2−) is independent on temperature, at 400 °C, the density dependence of G(CO2−) in the presence of N2O agrees well with that of {G(eaq−)+G(H)+G(OH)}." @default.
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• W1981845529 date "2008-10-01" @default.
• W1981845529 modified "2023-10-16" @default.
• W1981845529 title "Pulse radiolysis of sodium formate aqueous solution up to 400 °C: Absorption spectra, kinetics and yield of carboxyl radical CO2−" @default.
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• W1981845529 doi "https://doi.org/10.1016/j.radphyschem.2008.05.017" @default.
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