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- W1981863989 abstract "Abstract The nitrogenation of plutonium hydride powder (200–325 mesh) with nitrogen has been studied in the temperature range of 200–300°C. It was found that the nitrogenation obeyed the so-called linear law during an early period of the reaction and that the nitrogenation rate was not affected by gas flow velocity. It was also found that the rate increased with decreasing partial pressure of nitrogen, and was independent of the partial pressure of hydrogen. The activation energy was about 36 kcal/mol for PuH 3 and 47 kcal/mol for PuH 2 . X-ray diffraction study showed the product to be PuN, of which lattice parameter was 4·902 ± 0·002 A. From these results, it is considered that the nitrogenation is controlled by the reaction at the hydride-nitride interface. On the basis of the Langmuir isotherm, the dependence of the nitrogenation rate on the partial pressure of nitrogen is discussed." @default.
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- W1981863989 date "1974-11-01" @default.
- W1981863989 modified "2023-09-26" @default.
- W1981863989 title "Kinetic study of the nitrogenation of plutonium hydride with nitrogen" @default.
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- W1981863989 doi "https://doi.org/10.1016/0022-1902(74)80465-3" @default.
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