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- W1982000503 abstract "Pyrolysis experiments of isobutane, isobutylene, and 1-butene were performed over a temperature range of 550–750°C and a pressure of ∼0.8 atm. The residence time was ∼5 s. The fuel conversion and product selectivity were analyzed at these temperatures. The pyrolysis experiments were performed to simulate the gas-phase chemistry that occurs in the anode channel of a solid-oxide fuel cell (SOFC). The experimental results confirm that molecular structure has a substantial impact on pyrolysis kinetics. The experimental data show considerable amounts of C5 and higher species (∼2.8 mole % with isobutane at 750°C, ∼7.5 mole % with isobutylene at 737.5°C, and ∼7.4 mole % with 1-butene at 700°C). The C5+ species are likely deposit precursors. The results confirm that hydrocarbon gas-phase kinetics have substantial impact on a SOFC operation." @default.
- W1982000503 created "2016-06-24" @default.
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- W1982000503 date "2010-04-09" @default.
- W1982000503 modified "2023-10-17" @default.
- W1982000503 title "Kinetic Analysis of C4 Alkane and Alkene Pyrolysis: Implications for SOFC Operation" @default.
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- W1982000503 doi "https://doi.org/10.1115/1.4000677" @default.
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