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• W1982114461 abstract "A pressure-induced phase transition of FeOCl is discovered to occur at ${P}_{c}=15ifmmodepmelsetextpmfi{}1$ GPa. It is preceded by extremely anisotropic lattice compression, which is explained by a gradual collapse of the van der Waals gap between the chlorine atoms on the borders of the slabs of this layered compound. Single-crystal x-ray diffraction in a diamond anvil cell is used to show that the high-pressure phase can be described as a fourfold superstructure with monoclinic lattice distortion, described by a $4aifmmodetimeselsetexttimesfi{}1bifmmodetimeselsetexttimesfi{}2c$ supercell with space group $B{2}_{1}/m$ ($b$ unique). The high-pressure crystal structures have been used to uncover the mechanism of the phase transition, as the formation of alternating regions of increased packing density of chlorine atoms within a single layer and regions of interpenetrating layers. Raman and Mossbauer spectroscopies indicate that the phase transition is not related to electronic effects or magnetic order." @default.
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• W1982114461 date "2013-07-22" @default.
• W1982114461 modified "2023-10-07" @default.
• W1982114461 title "High-pressure behavior of FeOCl" @default.
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• W1982114461 doi "https://doi.org/10.1103/physrevb.88.014110" @default.
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