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- W1982378946 abstract "We report on the kinetics of electron transfer from an electrode in an electrochemical cell to zwitterviologen molecules. An unsymmetrical electron transfer mechanism is observed in the cyclovoltammogram. The charge transfer to the molecule is accompanied by a conformational change which causes an unusual switching characteristic. One and two electrons can be transferred to and from the zwitterviologen respectively, depending on the sweep rate of the electrochemical cycle. The relaxation into the ground conformation depends on the temperature. In situ ESR measurements allow for determination of the electron delocalization and spin counting. It will be shown, that spin 12 polaron as well as spinless bipolaron states can be created. Different mechanisms for the conformational changes will be discussed." @default.
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- W1982378946 date "1991-06-01" @default.
- W1982378946 modified "2023-10-11" @default.
- W1982378946 title "Electrochemical switching of zwitterviologen: A mechanism for molecular information storage" @default.
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- W1982378946 doi "https://doi.org/10.1016/0379-6779(91)91189-h" @default.
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