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- W1982482874 abstract "Abstract The effect of square-wave concentration-forcing operation on the rate of methanol production over two industrial catalysts was studied at 513 K and 2.86 MPa total pressure. Improvements as high as 25 percent relative to the optimal steady-state methanol production rate, in moles per gram catalyst per unit time, were obtained over BASF's S 3-85 catalyst. This occurred in a laboratory-scale fixed-bed reactor with gas mixing for a cycling time of τ = 12 seconds and for a cycle split relative to carbon monoxide of γCO = 0.20, the rest of the cycle being hydrogen. Improvements as high as 15 percent were also obtained over Imperial Chemical Industries ICI 51-2 catalyst, in a differential plug-flow reactor for τ = 24 seconds and γCO = 0.15. These improvements were obtained for pure-component steady cycling between carbon monoxide and hydrogen with a constant carbon dioxide molar concentration of 2 per cent (BASF catalyst) or 3 percent (ICI catalyst) present in both parts of the cycle. On the other hand,..." @default.
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- W1982482874 date "1994-01-01" @default.
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- W1982482874 title "AN EXPERIMENTAL STUDY OF CONCENTRATION FORCING APPLIED TO THE METHANOL SYNTHESIS REACTION" @default.
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- W1982482874 doi "https://doi.org/10.1080/00986449408936229" @default.
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