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• W1982638680 startingPage "1572" @default.
• W1982638680 abstract "Endohedral Cs@C60 molecules were formed by implanting low energy (E0=30–220 eV) Cs+ ions into C60 molecules adsorbed on gold. Both growth and etching experiments of the surface deposited C60 layer provide clear evidence for a submonolayer coverage. The Cs+ penetration and Cs@C60 ejection stages are shown to be a combined, single collision event. Thermal desorption measurements did not reveal any Cs@C60 left on the surface following the Cs+ impact. The Cs@C60 formation/ejection event therefore constitutes a unique example of a pick-up scattering by endocomplex formation. Kinetic energy distributions (KEDs) of the outgoing Cs@C60+ were measured for two different Cs+ impact energies under field-free conditions. The most striking observation is the near independence of the KEDs on the Cs+ impact energy. Both KEDs peak around 1.2 eV with similar line shapes. A simple model for the formation/ejection/fragmentation dynamics of the endohedral complex is proposed. The model leads to a strong correlation between the vibrational and kinetic energy of the outgoing Cs@C60. The KEDs are calculated taking into account the competition between the various decay processes: fragmentation and delayed ionization of the neutral Cs@C60 emitted from the surface, fragmentation of the Cs@C60+ ion, and radiative cooling. It is concluded that the measured KEDs are heavily biased by the experimental breakdown function. Good agreement between experimental and calculated KEDs is obtained." @default.
• W1982638680 created "2016-06-24" @default.
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• W1982638680 date "2004-01-13" @default.
• W1982638680 modified "2023-09-26" @default.
• W1982638680 title "The dynamics of endohedral complex formation in surface pick-up scattering as probed by kinetic energy distributions: Experiment and model calculation for Cs@C60+" @default.
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• W1982638680 doi "https://doi.org/10.1063/1.1632894" @default.
• W1982638680 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/15268284" @default.
• W1982638680 hasPublicationYear "2004" @default.
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