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- W1982685382 abstract "The approaching glass transition in polystyrene/toluene solutions leads to a sharp decay of both the collective diffusion coefficient $D$ and the thermal diffusion coefficient ${D}_{mathrm{T}}$ at concentrations above $0.2mathrm{g}/{mathrm{cm}}^{3}$. The Soret coefficient ${S}_{mathrm{T}}{phantom{rule{0ex}{0ex}}=phantom{rule{0ex}{0ex}}D}_{mathrm{T}}/D$ follows power-law scaling from semidilute to concentrated and is not influenced by the slowing down of the dynamics associated with the glass transition. Both $D$ and ${D}_{mathrm{T}}$ are governed by the same friction coefficient. The scaling behavior of ${S}_{mathrm{T}}$ with concentration on approach of the glass transition is compared to the divergence of ${S}_{mathrm{T}}$ near a consolute critical point." @default.
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- W1982685382 date "2002-04-22" @default.
- W1982685382 modified "2023-10-12" @default.
- W1982685382 title "Diffusion and Thermal Diffusion of Semidilute to Concentrated Solutions of Polystyrene in Toluene in the Vicinity of the Glass Transition" @default.
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- W1982685382 doi "https://doi.org/10.1103/physrevlett.88.185901" @default.
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