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- W1983303964 abstract "The heat capacity of a liquid in which monomers chemically react to form a macromolecule has been measured as the reaction progresses under isothermal conditions. It first irreversibly increases and then undergoes a step decrease to a value which is mainly due to vibrational contributions. This is remarkably similar to the decrease in heat capacity observed near the glass transition temperature on supercooling a liquid. The number of covalent bonds in the macromolecule's structure at its vitrification decreases with the decrease in the isothermal reaction temperature. Conclusions on the role of intra- and intermolecular interactions determining the molecular kinetics of liquids have been drawn." @default.
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- W1983303964 date "1993-12-01" @default.
- W1983303964 modified "2023-10-17" @default.
- W1983303964 title "Heat capacity change on isothermal vitrification during a macromolecule's growth" @default.
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- W1983303964 doi "https://doi.org/10.1016/0378-4371(93)90404-r" @default.
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