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- W1983606542 abstract "We introduce a new type of model that imitates polymer behavior of semiflexible polymers. In this model, the energy and entropy contributions to the free energy are treated as forces that act on the individual monomers, and thus guide the “movement” or “growth” of the chain. The model falls at the interface between theory and simulation, allowing statistical prediction of polymer conformational behavior of long polymer chains at a small computational cost. Results are compared with theoretical predictions by Spakowitz and Wang (SW) (Phys. Rev. Lett. 2003, 91, 166102) of the behavior of semiflexbile chain confined to the surface of a sphere and our own Monte Carlo simulations. The SW and Monte Carlo results are reproduced with the imitation model with surprising accuracy. The simple nature of the imitation model allows us to carry out calculations for very long chains, with which we show that the surface coverage of the sphere is a non-monotonic function of persistence length for a given fixed chain length..." @default.
- W1983606542 created "2016-06-24" @default.
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- W1983606542 date "2007-07-18" @default.
- W1983606542 modified "2023-09-25" @default.
- W1983606542 title "Vector Imitation Model of Semiflexible Polymers: Application to Polymer Adsorbed on a Spherical Particle" @default.
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- W1983606542 doi "https://doi.org/10.1021/ma062721+" @default.
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