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• W1983674071 abstract "A general theory is developed for the interaction of exctions with molecular vibrations in pure and impure molecular crystals. A study is made of a model Hamiltonian which describes the interaction of Frenkel excitons with harmonic oscillators, with particular attention paid to the case in which exciton bandwidth is fairly narrow. Equations of motion for molecular excitons are obtained in the form of Dyson equations using the method of double‐time Green's function. By solving the Dyson equations, it is shown that the vibrational energies of excitons in pure and impure molecular crystals, which can be classified into zero‐phonon and one‐phonon energies, are very different for different combinations of the energies of molecular vibrations and the exciton bandwidth. For example, a series of vibronic exciton bands is obtained for a pure crystal when the energies of phonons are larger than the exciton bandwidth while for an impure crystal, under certain circumstances, molecular vibrations can induce a delocali..." @default.
• W1983674071 created "2016-06-24" @default.
• W1983674071 creator A5064974506 @default.
• W1983674071 date "1967-04-01" @default.
• W1983674071 modified "2023-09-26" @default.
• W1983674071 title "Vibrational Properties of Excitons in Molecular Crystals" @default.
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• W1983674071 doi "https://doi.org/10.1063/1.1841073" @default.
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