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• W1984133098 abstract "Binary chromophore systems represent a new and very promising class of organic second-order nonlinear optical (electro-optic) materials, where favorable intermolecular electrostatic interactions lead to significantly enhanced electro-optic coefficients and to other favorable physical properties such as low optical loss and improved stability. In this report, laser-assisted poling of a binary chromophore system consisting of a photoaddressable chromophore host (DR-1-co-PMMA) containing a non-photoaddressable guest chromophore (YLD_124) is demonstrated. A factor of 2.5 enhancement in poling efficiency of the guest chromophore (compared to simple conventional electric field poling of the same material) is observed when polarized light is used to selectively enhance the order of the host chromophores. These results further emphasize the importance of favorable intermolecular interactions thought to exist between guest and host chromophores in binary chromophore containing materials. Thin-film samples were processed using an in situ reflection ellipsometry apparatus that was modified to perform real-time monitoring as well as to introduce 532 nm polarized laser light. Poled samples were then removed and the principal element of the electro-optic tensor, r33, was evaluated using the modified attenuated total reflection measurement method. Through the use of this approach, processing temperature, optical power, and electric poling field were optimized, and the dependence of resulting electro-optic properties on these variables was explored. Binary chromophore-containing materials may represent ideal model systems for studying intermolecular electrostatic interactions as well as realizing exceptionally large electro-optic activity and other photonic and electronic properties dependent on noncentrosymmetric (acentric) order." @default.
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• W1984133098 date "2008-05-01" @default.
• W1984133098 modified "2023-09-30" @default.
• W1984133098 title "Laser-Assisted Poling of Binary Chromophore Materials" @default.
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• W1984133098 doi "https://doi.org/10.1021/jp712154g" @default.
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