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- W1984138659 abstract "Abstract A new low-coverage (up to 10% of monolayer) adsorption isotherm is developed from a statistical thermodynamic derivation. This low-coverage polyomino (LCP) isotherm is similar to the two-dimensional van der Waals (VDW) isotherm. However, in the VDW isotherm the lateral interaction term has a linear dependence on the surface coverage, θ; whereas, in the LCP isotherm higher order terms are present. The effect of these additional θ terms on the isotherm is shown. The LCP model takes into account the structure and distribution of random adatom clusters formed on the surface. The LCP isotherm is based on separating the canonical partition function for the lattice gas into molecular partition functions which are classified according to the number of nearest neighbors surrounding an adatom. This partition scheme depends on information obtained from percolation theory on the sizes and shapes of adatom clusters (polyominoes) as a function of surface coverage on a triangular lattice." @default.
- W1984138659 created "2016-06-24" @default.
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- W1984138659 date "1985-10-01" @default.
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- W1984138659 title "Low-coverage polyomino adsorption isotherm" @default.
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- W1984138659 doi "https://doi.org/10.1016/0021-9797(85)90207-3" @default.
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