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- W1984156950 abstract "Three novel ring-like compounds formulated as [Ln(Phtfac)3(NITpPy)]2 (LnIII = Gd 1, Tb 2, Dy 3; HPhtfac = 4,4,4-trifluoro-1-phenylbutane-1,3-dione; NITpPy = 2-(4-pyridyl)-4,4,5,5-tetramethyl-4,5-dihydro-1H-imidazolyl-1-oxyl-3-oxide) were synthesized and structurally and magnetically characterized. Three compounds possess cyclic dimer structure in which each pyridine substituted radical links two different metal ions through the oxygen of nitroxide group and the pyridine nitrogen. DC magnetic studies show the Ln(III) ion interacts ferromagnetically with the directly bonding nitronyl nitroxide. Both Tb(III) and Dy(III) clusters show frequency-dependent ac magnetic susceptibilities, indicating single-molecule magnet behavior. It is demonstrated that the β-diketonate coligand may play an important role in determining the magnetic relaxation for the lanthanide-radical system." @default.
- W1984156950 created "2016-06-24" @default.
- W1984156950 creator A5006182005 @default.
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- W1984156950 date "2012-01-01" @default.
- W1984156950 modified "2023-10-17" @default.
- W1984156950 title "Modulating spin dynamics of cyclic LnIII-radical complexes (LnIII = Tb, Dy) by using phenyltrifluoroacetylacetonate coligand" @default.
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- W1984156950 doi "https://doi.org/10.1039/c2dt11671e" @default.
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