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- W1984492010 abstract "Core-level 4${mathit{f}}_{7/2}$ photoemission spectra have been measured from a single, bifacial W crystal, which has both a flat W(110) and a vicinal, stepped W(110) [W(320)] surface. This procedure reduces uncertainties in the quantitative description of peaks in the spectra from W(320). Various analyses, including nonlinear least-squares curve fitting, show that the average surface core-level shift (SCS) for W(320) is only ensuremath{sim}-140 meV, compared to -310 meV for W(110) and that, at a maximum, only two of five terrace rows are isoelectronic to W(110) surface atoms. The absence of a large SCS for the step-edge atoms contradicts earlier interpretations of W(320) core-level spectra and departs significantly from expectations based on atomic-coordination models or tight-binding calculations of a bulk truncated surface. We suggest that systematic errors are responsible for the differences in reported core-level shifts for W(320). Implications of possible step-edge-driven atomic rearrangements are discussed." @default.
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- W1984492010 date "1994-11-15" @default.
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- W1984492010 title "Surface core-level shifts and atomic coordination at a stepped W(110) surface" @default.
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- W1984492010 doi "https://doi.org/10.1103/physrevb.50.14481" @default.
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