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• W1984558730 startingPage "3648" @default.
• W1984558730 abstract "Starting from an ab initio intermolecular potential, we have calculated the mean field states for the librations in the ordered α and γ phases of solid N2, using a basis of spherical harmonics up to lmax=12. The correlation between the mean field solutions was then taken into account via a libron model based on the random-phase approximation or time-dependent Hartree method. The calculated librational frequencies are rather accurate, showing that the discrepancies in earlier results with the ab initio potential are mainly due to the breakdown of (quasi-)harmonic models for the librations, even in the ordered phases." @default.
• W1984558730 created "2016-06-24" @default.
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• W1984558730 date "1984-10-15" @default.
• W1984558730 modified "2023-09-26" @default.
• W1984558730 title "<i>A</i><i>b</i> <i>i</i><i>n</i><i>i</i><i>t</i><i>i</i><i>o</i> description of large amplitude motions in solid N₂. I. Librons in the ordered α and γ phases" @default.
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• W1984558730 doi "https://doi.org/10.1063/1.448114" @default.
• W1984558730 hasPublicationYear "1984" @default.
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