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- W1984906294 abstract "A finite-difference time-domain formalism for simulating coherent linear pulse propagation is presented that incorporates a medium response described by any two-time energy gap correlation function. Two algorithms, for real and complex correlation functions, are developed to evaluate the electric polarization through explicit treatment of the density matrix for a two-level system. The coherence relaxation terms in the resulting finite-differenced Maxwell–Liouville equations depend on integrals over the energy gap fluctuation correlation function. The algorithms are used to simulate ultrashort mid-infrared pulse propagation through optically dense samples of HDO in liquid D2O as a demonstration of their performance and flexibility. These algorithms represent a first step toward the goal of incorporating complicated material responses into the full-field simulation of nonlinear pulse propagation and nonlinear optical spectroscopy." @default.
- W1984906294 created "2016-06-24" @default.
- W1984906294 creator A5011786727 @default.
- W1984906294 date "2003-07-02" @default.
- W1984906294 modified "2023-09-24" @default.
- W1984906294 title "Correlation function-based finite-difference time-domain method for simulating ultrashort pulse propagation. I. Formalism" @default.
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- W1984906294 doi "https://doi.org/10.1063/1.1580804" @default.
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