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• W1984942490 endingPage "1975" @default.
• W1984942490 startingPage "1971" @default.
• W1984942490 abstract "Molecular dynamics simulations of rigid, defect-free single-walled carbon nanotubes have previously suggested that the transport diffusivity of gases adsorbed in these materials can be orders of magnitude higher than any other nanoporous material (A. I. Skoulidas et al., Phys. Rev. Lett. 2002, 89, 185901). These simulations must overestimate the molecular diffusion coefficients because they neglect energy exchange between the diffusing molecules and the nanotube. Recently, Jakobtorweihen et al. have reported careful simulations of molecular self-diffusion that allow nanotube flexibility (Phys. Rev. Lett. 2005, 95, 044501). We have used the efficient thermostat developed by Jakobtorweihen et al. to examine the influence of nanotube flexibility on the transport diffusion of CH4 in (20,0) and (15,0) nanotubes. The inclusion of nanotube flexibility reduces the transport diffusion relative to the rigid nanotube by roughly an order of magnitude close to zero pressure, but at pressures above about 1 bar the transport diffusivities for flexible and rigid nanotubes are very similar, differing by less than a factor or two on average. Hence, the transport diffusivities are still extremely large compared to other known materials when flexibility is taken into account." @default.
• W1984942490 created "2016-06-24" @default.
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• W1984942490 date "2006-01-12" @default.
• W1984942490 modified "2023-10-17" @default.
• W1984942490 title "Transport Diffusion of Gases Is Rapid in Flexible Carbon Nanotubes" @default.
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• W1984942490 doi "https://doi.org/10.1021/jp056911i" @default.
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